When studying ferrofluidic flows, as one example of magnetic flow dynamics, in terms of instability, bifurcation, and properties, one quickly finds out the additional challenges magnetic fluids introduce compared to the investigation of “classical”, “ordinary” shear flows without any kind of particles. Approximation of ferrofluids as fluids including point-size particles or, more realistic fine size particles, the relaxation times of the magnetic particle, their interaction between each other, i.e., the agglomeration and chain forming effects, and the interaction/response between any external applied field and the internal magnetization are just few examples of challenges to overcome. Further dependence on the considered model system, the direction of the external applied magnetic field (homogeneous or inhomogeneous) is crucial, as it can break the system symmetry and thus generate new solutions. As a result, the classical Navier–Stokes equations become modified to the more complex ferrohydrodynamical equation of motion, incorporating magnetic field and magnetization of the fluid itself, which typically makes numerical simulations expensive and challenging. This chapter provides an overview of the tasks/difficulties from describing and simulating magnetic particles, their interaction, and thus finally resulting modification in rotating flow structures and in particular instabilities and bifurcation behavior.
- magnetic fluid
- complex system
- growth rate
- finite-size effect
- internal magnetic field
- particle interaction
- elongational flow
Ferrofluids  represent one example of magnetic particles with a variety of applications, ranging from liquid seals in rotating systems, their use in computer hard drives, as well as in laboratory experiments, to study geophysical flows [2, 3]. However, deeper fundamental study of their magnetohydrodynamics is inevitable, as there are many modeling assumptions that have been implemented to make theoretical descriptions tractable. Ferrofluids are manufactured fluids which consist of dispersions of magnetized nanoparticles in various kinds of liquid carriers. Stabilizing against agglomeration is typically achieved by the addition of a surfactant monolayer onto the magnetic particles. Being no magnetic field present, the magnetic nanoparticles are randomly orientated, which results in a zero-net magnetization of the fluid. Only effect of the present nanoparticles is a typically small alteration to the fluid’s density and viscosity. Applying a sufficiently strong magnetic field, the ferrofluid flows toward certain regions of the magnetic field. The hydrodynamics of the system can be significantly changed, and properties of the fluid, e.g., the viscosity, are altered. Therefore, nowadays, they are widely used by various car manufactures in order to provide adaptable suspensions, i.e., changing the damping characteristics of an antishock/damper due to modified viscosity of the ferrofluid under influence of an external applied magnetic field. Both numerical simulations and experiments show that any applied magnetic field, whether radial, axial, azimuthal, transversal, or any combination of the previous stabilizes the basic state [4, 5, 6, 7, 8, 9]. This stabilization effect depends, among others, on the particle-particle interactions of the fluid . A strong interaction leads to large/crucial changes in flow behavior, which are driven by the formation of internal flow structures. While an axisymmetric field leaves the flow structures untouched (compared to classical Couette flow), a finite transverse, in-plane magnetic-field component breaks axisymmetry, enforcing new nonlinear effects, modify present flow structures, and can produce new flow structures.
Among various others, one important point to look at is the applied magnetic field, in particular its characteristics while penetrating a moving ferrofluid. In order to describe the hydrodynamics of ferrofluids in containers/boxes typically, models are used which assume that the internal magnetic field and the external applied magnetic field are equal [4, 5, 6]. However, such a simplification is only a leading order approximation, as the magnetic field in the container typically is modified, based on the magnetic susceptibility of the ferrofluid. First work trying to account for modifications  includes an expression for the angular velocity of the ferrofluid particles, which differs from the ferrofluid itself due to the magnetic torques acting on the particles. The results are significant differences from the external field, providing among others, a much changed body force in the governing equations. More concretely, the interaction between a uniform external field and the susceptibility of the ferrofluid-filled annulus can be shown to result in a field with an radial dependence superimposed on the external field.
Further common assumption when describing the hydrodynamics of magnetic particles as ferrofluids is to consider them as point-wise objects and ignore their finite size and specific properties. However, in real, such particles typically aggregate to form clusters having the form of chains, and thus they hinder the free flow of the fluid and increase the viscosity [9, 10, 11], and change their rheology and transport properties . In this type of structure’s formation, it is also assumed that the interaction parameter is usually greater than unity , and thus the strength of the grain-grain interaction can be measured in terms of the total momentum of a particle. Regarding the magneto-dissipative structure of ferrofluid dynamics, one can derive, based on general principles, an equation for macroscopic ferrofluid dynamics. The magnetization’s relaxation equation includes an additional term that is proportional to the product of the magnetization’s magnitude and the symmetric part of the velocity gradient tensor, which can describe an elongational flow scaled by a so-called transport coefficient . Such description also exists in the dynamics of nematic liquid crystals, as the flow alignment modifies the director field in an applied shear flow .
It is worth to mention that there are further crucial and important considerations for describing ferrofluids and in general fluids with magnetic particles which are also important as the discussed ones. However, these are not considered in the present chapter. Therefore, we refer to the huge amount of literature, which can be essentially found by the presented references. Two prominent examples of these further considerations are the modulation of the relaxation times of magnetic particles [7, 13], e.g., Neel’s or Braun’s and the consideration of monodisperse vs. polydisperse materials [7, 17, 18].
In this chapter, we will consider a rotating ferrofluid in Taylor-Couette geometry. First, we are going to describe the modifications in flow solutions and its structural properties and alterations in primary supercritical bifurcation thresholds induced/forced by an external applied magnetic field. Following, we will discuss two different approaches to come to a more realistic description of ferrofluidic flows. Therefore, we will modify and extend the basic ferrohydrodynamical equations. First, considering a modification of the internal magnetic field, which differs from the external applied one due to its internal magnetization. Second incorporating elongational flow. The latter aims to consider finite size effects of the magnetic particles, as well as agglomeration and chain formation procedures.
2. System and theoretical description
As a prototypical system to investigate the influences of a magnetic field on a rotating ferrofluid system, we consider Taylor-Couette flow (Taylor Couette system, TCS) [19, 20] driven by the independent differential rotation of two concentric cylinders (Figure 1).
The inner cylinder of radius rotates at , and the outer cylinder of radius rotates at . If not other stated, in this chapter, periodic boundary conditions are considered in the axial direction with periodicity of length and no-slip boundary conditions on the cylinder walls. The system is described using a cylindrical polar coordinate system with a velocity field . The radius ratio of the cylinders is , and the aspect ratio is . The gap between the cylinders is filled with a viscous, incompressible, and isothermal ferrofluid. An external homogeneous magnetic field is applied, where is the transverse direction and is the axial direction, respectively (Figure 1).
The flow dynamics of an incompressible homogeneous monodisperse ferrofluid with kinematic viscosity and density is governed by the incompressible Navier–Stokes equations, including magnetic terms and the continuity equation. Following, an approach based on the model of Niklas [4, 5] is used, where the magnetic fluid is assumed to be incompressible, nonconducting, and to have a constant temperature and a homogeneous distribution of magnetic particles. Using the gap as the length scale, the diffusion time as the time scale, scaling pressure with , the magnetic field , and the magnetization with (is the magnetic constant, i.e., magnetic permeability of free space), the nondimensional governing equations are
The cylinders are considered to be of no-slip type with velocity boundary conditions
where the inner and outer Reynolds numbers are and , respectively.
2.1 Magnetization equations
In order to solve (1), one needs additional information about the magnetic particles themselves, in particular their properties and interaction with an applied magnetic field. Therefore, (1) is solved together with an equation that describes the magnetization of the ferrofluid. A first approximation is to use the equilibrium magnetization of an unperturbed state with a homogeneously magnetized ferrofluid at rest with the mean magnetic moments orientated in the direction of the magnetic field, , where is the magnetic susceptibility of the ferrofluid, determined using Langevin’s formula . The ferrofluid considered for all simulations in this chapter is APG933  with . However, a ferrofluid’s magnetization is also influenced by the flow field. For the presented numerical simulations, an approach based on the model of Niklas [4, 5, 6] is used. Furthermore, a stationary magnetization near equilibrium considering a small perturbation at the equilibrium magnetization and small relaxation times , where is the absolute value of half of the vorticity and is the magnetic relaxation time. In the near-equilibrium approximation, Niklas  determined the relationship between the magnetization , the magnetic field , and the velocity to be
with being the vorticity and the Niklas coefficient
where is the dynamic viscosity and is the volume fraction of the magnetic material.
2.2 Ferrohydrodynamic equations of motions
The magnetization can be eliminated from (1) by using (3) in order to obtain the ferrohydrodynamic equation of motion :
where and are the dynamic pressure incorporating all magnetic terms which can be written as gradients. Note that the relaxation time could typically be defined by , where is the Brownian relaxation time and is the averaged diameter of the magnetic particles. For simplicity, to investigate the different effects, i.e., internal magnetization and elongational flow (see below), we assume that is constant, which is independent of the magnetic field . The considered relaxation time is based on the experimental result  .
Consider external field to be equal to internal one , (5) can be simplified to
In this approach, the magnetic field and all the magnetic properties of the ferrofluid influence the velocity field only via the magnetic field, the Niklas parameter [4, 5, 6], whereby magnetic field strengths are:
In this approach, and are dimensionless numbers, describing the strength of the applied magnetic field.
3. Ferrofluidic flow under finite magnetic field
3.1 Introduction and motivation
We start our discussion with the investigation of the influence of a homogeneous magnetic field on a ferrofluid. In this first part, we will assume that the internal magnetic field is equal to the external applied magnetic field, i.e., homogeneous. Moreover, we ignore in this section any kind of finite size effects, e.g., possible agglomeration and chain formation, later considered as elongational flow effect (Section 4). Therefore, we consider the ferrofluid particles as point-size objects without any 3D expansion. Structure, dynamics, symmetry properties, bifurcation, and stability behavior of different vortex structures are investigated for axial and transversal magnetic fields, as well as combinations of them, i.e., oblique magnetic field. We will see that a transversal magnetic field has significant influence. It modulates and changes the classical flow structures, as well the basic state (Circular Couette flow, CCF) as the classical primary supercritical ones, Taylor vortex flow (TVF) and the spiral vortex flow (spirals, SPI). They are replaced by wavy-modulated flow structures: wavy Taylor vortex flow (wTVF) and wavy spiral vortex flow (wSPI), as well as they forward bifurcate out of the modified 2-fold circular Couette flow (2-CCF).
3.2 Flow structures
3.2.1 Flow structures in absence of a magnetic field
There are two fundamental basic, topologically different flow structures appearing in (classical) Taylor-Couette flow (see also Nomenclature and abbreviations section). These are either toroidally closed Taylor vortices (Taylor vortex flow, TVF) and helical spiral vortices (spiral vortex flow/spirals, SPI) . Figure 2 shows the structure of these fundamental solutions, TVF and SPI (here for a left-handed SPI with azimuthal wavenumber ), by using isosurfaces of the azimuthal vorticity. Because of the system symmetry , we only discuss left-handed SPI. Without other parameters, e.g., axial through flow, left- and right-handed SPI are mirror images of each other. These pure states can also be found modulated as wavy structures, which are topologically identical with the pure states. However, they show a wavy-like deformation that results from additional and other stimulated modes compared to the classical solutions.
While classical wavy flow solutions [27, 28, 29, 30, 31, 32, 33, 34, 35, 36] are well known and have already been widely discussed in literature regarding TCS, the ones generated by a magnetic field are different. In particular, the magnetically induced wTVF are nonrotating structures having a pinned phase, contrary to the classic wTVF, which rotate azimuthally. Regarding the flow structure, the imposed magnetic field shrinks and expands the vortices at different cross sections of constant , resulting in an azimuthal alternating wide and narrow vortex belly structure.
3.2.2 Flow structures—mode coupling in magnetic fields
Following, we will have a quick look at the impact on the different applied magnetic field with respect to the flow structures and in particular their mode spectra. The modifications in NSE due to the additional terms incorporating magnetization and magnetic field result in various new phenomena. Most important is probably the fact that magnetic fields with a finite transversal component stimulate additional modes. Depending on different external applied magnetic fields, Figure 3 presents a schematic plot for the different stimulated modes, depending on the applied field.
Having a pure axial field applied the mode spectra, the flow structures remain qualitatively similar to the no field (N) case (Figure 3(a)). A TVF still contains only the axisymmetric modes (with dominant n = 1, see also Figures 2 and 6). Similarly, L1-SPI, i.e., a left-handed SPI flow with azimuthal wavenumber contains modes only on the diagonal (with dominant , see also Figures 2 and 6). However, if a field with finite transversal component is applied additional mode become finite and the flow structures change. A pure transversal field excites modes lying on the secondary diagonal (Figure 3(b)). Thus, as a result, the pure states of TVF and SPI vanish in the presence of a transversal magnetic field. They become wavy-like modified, resulting in wTVF and wSPI. Finally, having a magnetic field with either axial and transversal component , there are further interactions, which result in stimulation of additional modes (Figure 3(c)). Moreover, these additional modes can induce further nonlinear mode couplings. As a result, the mode spectra contain more nonzero components (Figure 3(c) and Figure 6 for numerical results). Thus all flow structures in a magnetic field with transversal component differ qualitatively from the classical flows found in the absence of magnetic fields [6, 26].
3.3 Effect of finite magnetic fields
3.3.1 Basic state and symmetries
If only a pure axial magnetic field, (see Figure 1), the classical circular Couette flow (CCF) is observed, with , where , and , is a solution of (5) as the associated vorticity is parallel to the applied magnetic field and therefore all magnetic terms vanish. Although for magnetic fields that are orientated purely in the radial or azimuthal direction, the basic state changes but remains axisymmetric with deviations from CCF only having an azimuthal component [4, 23]. As a result, in all of these cases, the basic state is invariant to a number of symmetries (azimuthal rotation, mirror symmetry, and axial translation) whose actions on a general velocity field are
On the contrary, for a field with a finite transverse component, the base state is no longer axisymmetric. Although the basic state remains invariant to and a modified mirror symmetry , a transverse magnetic field T breaks the continuous axisymmetry , resulting in a basic state with discrete symmetry , i.e., with azimuthal wavenumber . Following, we will refer to this modified 2-fold symmetric CCF as 2-CCF. It is important to mention that this state is stationary , which is in contrast to the generic breaking of a symmetry which would result in a rotating wave.
3.3.2 Bifurcation behavior
As seen in Section 3.2, an applied magnetic field can stimulate additional modes and thus changes the Fourier mode spectrum of flow structures resulting in new solutions. The results are wavy-like modified flow states. It is to expect that these mode-stimulated modifications also influence and appear in the primary bifurcation thresholds of the solutions, as well as in their growth rate. Following, we will have a look at the bifurcation behavior of the different flow structures with the additionally field-induced modes explained in Section 3.3. In particular, we will focus on four different field configurations: no field (N) ; pure axial field (A) ; pure transversal field (T) ; and oblique field (O) ((7) for parameters ).
Considering these four, non, pure axial, pure transversal, and oblique magnetic fields, Figure 4 illustrates the stable forward bifurcating branches of toroidally closed TVF and of wTVF solutions, respectively. Figure 5 shows the bifurcation diagrams for helical SPI and wSPI in an analogous way. Note that the shown wavy-like modulated flow states only result from symmetry breaking due to finite transversal field component. In the Figures 4 and 5, the relative distance is used as control parameter for easier comparison of the bifurcation branches (stands for the critical onset Reynolds number of the flow structure, which depends on various system parameters. These are the aspect ratio , the radius ratio , the outer Reynolds number , axial boundary conditions, and the field strength , , respectively). The main reason to use is the shift in the bifurcation onset, which varies depending on the applied field direction.
Displayed in the Figures 4 and 5 are the moduli of the dominant, as well as the first higher harmonic modes of the corresponding structure (see Appendix (18) and (19)), e.g. and for TVF. Furthermore, the largest field-induced mode amplitudes and (only in oblique configuration) of the wavy structures (cf. schematics in Figure 3) are included for comparison.
Axial field (A): As a pure axial magnetic field does not stimulate any further modes within the mode-spectra (Figure 3(a)), the flow states TVF and SPI and their structural properties remain qualitatively similar, and they are as without a field. However, quantitative, they eventually change. First important effect is the rise of the onsets to higher values of [6, 7]. Thereby, the upward shift depends on the various system control parameters (e.g., ). For parameters in Figure 4, the onset of TVF rises by about 25%, and for the parameters of Figure 5, the SPI bifurcation threshold moves upward in by about 15%. For the latter, consequently also corresponding SPI frequencies are increased in an axial field. Other change regarding Figure 4 is the amplitude of the modes with increasing the parameter (weakest for nonfield and strongest for oblique field configuration).
Transversal field (T): A transversal magnetic field stimulates additional azimuthal modes (Section 3.2) as illustrated in Figure 3(b). Thus, based on this knowledge, one can already expect a more dramatic influence on the classical TVF and SPI structures. As a pure axial field, a transversal field also delays the onset of the primary bifurcating structures, i.e., it stabilizes the basic state. Furthermore and more important is the fact that such a field also changes the flow structural properties in qualitative manner. The growth of the additional modulus (18) (for toroidally closed flow states) with changes the pure TVF to a wavy-like modulated wTVF. Analog pure SPI changes to wSPI (shown for L1-(w)SPI in Figure 5) due to the additional (see Figure 3(b)), indicated by the growth of the modulus in Figure 5. It is worth to mention that due to the mode stimulation and interaction, also the (1,-1) mode becomes excited, which is similar to structure R1-(w)SPI. Note, the same also holds for the symmetry-related mirror image L1-(w)SPI.
Thus, in the presence of a magnetic field with a finite transversal component, the pure/classical TVF and SPI structures are modified. They are replaced by their wavy-like counterparts, wTVF and wSPI, which now bifurcate as primary structured solutions forward out of the CCF-2 ground state; note that already the basic state has an additional mode-2 symmetry due to the symmetry-breaking effect of the transversal field and as such already differ from the classical CCF (Section 3.3.1). As for axial field, the magnitude of stabilization varies with given system control parameters. In general, it is slightly smaller compared to the stabilization effect of an axial field. For instance for parameters presented in Figures 4 and 5, the upward shift for the onset of wTVF (wSPI) is about 20% (12%) in an axial (transversal) magnetic field.
Important to mention that a finite transverse component breaks the system symmetry but does not change the degeneration between left- and right-handed SPIs. Both solutions keep bifurcating at the same critical values. The latter is different to the effect of an axial flow, for instance. Aside that such a flow also breaks the system symmetry, it separates both left- and right-handed SPI solutions. Under axial applied flow, they appear at different critical values.
Oblique field (O): As already seen for both pure field configurations, either or , the onset of (w)TVF and (w)SPI is shifted to higher values. In fact in a field, obliquely orientated to the cylinder , the magnitude of shift is bigger compared to the pure cases. In addition, as discussed before, such a superposition of an axial and a transversal field stimulates also new, additional modes with higher mode index combinations (Figure 3(c) and for numerical simulations Figures 4(c,d), 5(c,d), and 6(e,f)).
A common finding for (w)TVF and (w)SPI is that their dominant mode amplitudes for (for (w)TVF) and (for (w)SPI) grow with respect to the bifurcation onsets. Although the absolute value depends on the different applied magnetic field, comparing the moduli at the same relative distance from the respective onset (Figures 4 and 5, compare dominant mode amplitudes), one finds the following relations
For helical flow structures, the larger variety of mode interactions due to the basic spectra (e.g.  for pure L1-SPI [R-SPI]) results in significant variation of the higher order and secondary stimulated modes, depending on the field configuration (see in particular Figures 3(c), 4(d), and 5(d)).
Based on the both bifurcation diagrams presented in Figures 4 and 5, it is worth to remind that in the case of a finite transversal field component , no pure solutions, TVF and SPI, exist. They become replaced by wavy-like modulated wTVF and wSPI. However, independent of the field, leading mode amplitude of the respective flow state, (w)TVF and (w)SPI, follows a typical square-root forward bifurcation, whereby the slope of its square grows with the applied field strength.
3.3.3 Vortex structures and mode contents
Having discussed the changes that different oriented magnetic fields can cause in the bifurcation behavior and mode stimulation of (w)TVF and (w)SPI, respectively, one can imagine that these also coincide with flow structural modifications. Now, we will address these structural changes of the vortices and the associated changes in the mode contents of the flows in more detail.
Figure 6 shows isosurfaces of the azimuthal vorticity over two axial wavelengths (for visual purpose) for supercritical flow states (w)TVF and (w)SPI in the three different considered field configurations: (a,b) no field applied (N), (c,d) pure transverse field (T), and (e,f) oblique field (O) at parameters and as indicated.
A good quantity in order to visualize the field induced changes in the 3D vortex structures are isosurfaces of the azimuthal vorticity . These surfaces appropriately convey structural details of the vortex flows in question .
Axial field (A): As a pure axial field does not break any continuous symmetry of the system, there is neither qualitative change in the structure of TVF and SPI in real space nor the mode structure of the flow in the Fourier plane (not shown, but similar as Figure 2(a,b); only quantitative the mode amplitudes are slightly larger). TVF still consists of toroidally closed, rotationally symmetric vortex tubes with a mode spectrum containing only modes (Figure 2(a)). And also, the helically oriented, open vortex tubes of SPI (here for left-winding spiral L-SPI) containing modes as shown in Figures 2(b) and 3 (mirror image of right-winding R-SPI analog) are unaffected by an axial field.
Transversal and oblique field (T, O): Having a magnetic field with finite transversal component crucially changes the scenario as TVF, and SPI structures are replaced by modified flow states due to the presence of such a magnetic field. In general, the isosurfaces become wavy-like deformed, and additional Fourier modes are stimulated as described before (Section 3.3; see also schematics in Figure 3). For pure transversal field, this mode stimulation results in wTVF with additional modes aside the (Figure 6(c)) and in wSPI with modes on the secondary diagonal(s) in addition to the SPI modes on the diagonal (Figure 6(d)). Beyond these, an oblique field further stimulates the modes in wTVF and in wSPI due to more complex nonlinear dynamics/mode interaction. In particular, the spatio-temporal properties of the wTVF generated due to symmetry breaking magnetic field, either transversal or oblique (Figure 6(c,e)), differ significant from those of the classic wTVF. The structure of classical wTVF rotates as a whole in azimuthal direction [27, 32, 33, 34, 35].
The wavy-like deformation on the toroidally closed vortices introduced by a magnetic field with a finite transversal component is different. Regarding Figure 6(c,e), one sees that the tubes of isosurfaces of the azimuthal vorticity become strong modified and bent at certain azimuthal cross sections of constant in comparison with the pure TVF tubes. Classic wTVF arises by deforming the TVF such that the axial stack of closed vortex tubes is wave-like modulated, bending axially upward and downward. Then, this deformation structure of the vortices rotates as a whole with a characteristic frequency. In contrast to these classical rotating wTVF, the wTVF initiated due to the symmetry-breaking transversal field component is stationary and does not rotate in azimuthal direction, instead, developing an 2-fold belly structure. It is worth to mention that such 2-fold symmetry also applies to the basic state. Thus, the classical rotational, axisymmetric CCF is replaced by the 2-CCF due to the symmetry breaking in the transversal magnetic field (see Section 3.2).
Consider wSPI, one can identify qualitative similar wavy characteristics, whereby the topological differences are weaker in comparison to wTVF. As the classical SPI structures already rotate without magnetic field, this also remains for wSPI in the presence of magnetic fields. However, also wSPI remains structural almost identical, and their modulation amplitude becomes enforced at certain cross sections of constant in presence of a transversal field component.
The basic state (CCF) loses stability either to (w)TVF (Figure 5) or (w)SPI (Figure 6). In case of wTVF, a supercritical pitchfork of revolution bifurcation breaks the axial translational symmetry (8.3) and parameterizes the axial location of the steady axisymmetric family of solutions. On the other hand, (w)SPIs appear in a supercritical Hopf bifurcation which breaks the mirror symmetry (8.2), resulting in a pair of symmetrically related spiral states, one with left-handed and the other with right-handed winding. It is worth to mention that a finite transverse magnetic field T breaks the axisymmetry , resulting in a basic state with discrete symmetry , i.e., with azimuthal wave number (section 3.3.1). Note that this state is stationary, which is in contrast to a generic breaking of an symmetry, resulting in a rotating wave.
3.3.4 Stabilization of basic state: point of higher co-dimension
For TCS, a crucial point of special interest in the phase diagram is the bicritical, co-dimension two point, , at which the primary bifurcation thresholds of TVF and SPI intersect/converge and as thus exchange the stability of the primary bifurcating solution . For instance, in absence of a magnetic field and given wavenumber , the -point is given by and  (Figures 7(a) and 8(a)); for smaller (stronger counter-rotation), SPI bifurcate stable, and for larger (less counter-rotation and co-rotation), TVF bifurcate stable respectively with increasing (Figure 8(a)). Thus, with increasing , the 2nd solution bifurcates as unstable solution. Note that the -point is quite sensitive to the axial wavenumber; for different , it moves toward higher and smaller . This bifurcation scenario also holds for wTVF and wSPI in oblique and transversal magnetic fields.
It is worth to mention that the curves in Figures 7(a) and 8 present “marginal stability” thresholds. These are obtained for a fixed wavenumber , which differ from the ‘critical’ thresholds. The latter is defined by the (smallest) Reynolds number, for which the flow structure first appears, which crucially depends on . Thus, the intersection points of the curves for TVF and SPI (e.g., Figure 7(a)) are critical values, with respect to the fixed wavenumber.
Figure 7(a) illustrates an example for the influence of different axial magnetic field strength on the bifurcation thresholds for TVF and SPI and the variation on the location of this bicritical point. These are results of linear calculations and were obtained with a shooting method . Solid blue (dashed orange) lines refer to TVF (SPI). Note that always the lower (in ) bifurcating vortex solution is stable and the upper one is unstable. As discussed in Section 3.2, increasing stabilizes the CCF basic state, both, against TVF and SPI, i.e., the upward shift of the respective threshold curves. In general, the strength of the stabilization effect is larger for helical SPI vortex structures than for toroidally closed TVF (e.g. Figure 8). As a result, the -point moves toward more negative (i.e., toward the left in Figure 7(a)). Thus, it is observed that the region of primary, stable bifurcating TVF expands with increasing .
The same scenario also applies for transversal and oblique magnetic field configuration, whereby the magnitude of the shift is biggest for a pure axial magnetic field and almost equal for a pure transversal and oblique magnetic field (slightly larger for the latter). Figure 7(b,c) displays the bifurcation thresholds for fixed outer cylinder rotations, and with increasing , resulting from fully nonlinear simulations. The slopes in Figure 7(b,c) depend crucially on . However, in general, the slopes for SPI are steeper than for TVF. For small to moderate field parameters, TVF is the primary stable bifurcating structure while SPI bifurcate secondarily and unstable. For stronger fields, the structures interchange stability and bifurcation order.
Summarizing, for fixed , an axial field shifts the onset of helical SPI more strongly than the one of toroidally closed TVF. We furthermore found this behavior to appear for all parameters and magnetic fields: either for axial, transversal, and oblique magnetic fields (Figure 8). In this case, that for transversal and oblique fields, all structures are wavy-like modulated; wTVF and wSPI, respectively (see also Section 3.2).
In pure axial or pure magnetic fields, the upward shifts of the bifurcation values, the stabilization of the basic state (CCF or 2-CCF), i.e., the onset of the primary stable flow state (w)TVF or (w)SPI grows linearly (Figure 7(b,c)) with the squared magnetic field parameters or , respectively . Thereby, the magnitude of stabilization shift depends crucially on , in general is largest close to outer cylinder at rest.
3.3.5 Marginal stability thresholds: Stabilization of the basic state
Before going into detail about the stabilization of the basic state it is worth, once more to mention, that the basic state can be different in presence of a magnetic field, whether the field contains a symmetry breaking transversal component or not. For pure axial field, one finds the classical CCF which becomes replaced by the 2-fold symmetric 2-CCF for fields with finite transversal component (see also Section 3.3.1).
Figure 8 presents bifurcation thresholds for vortex flows under the influence of different magnetic fields. Shown is the diagram, along which the CCF state loses stability. For comparison, (a) shows the thresholds in absence of any field , while the same thresholds are shown for (b) a transversal , (c) an axial , and (d) an oblique field . These results were obtained by nonlinear simulations with the full field ferrohydrodynamical Eqs. (11), considering a short periodic TCS with . See also Figure 7, for linear stability analysis, in which the shift of the higher co-dimension -point is shown together with stabilization of CCF in an axial field.
For all bifurcation thresholds of TVF, SPI, wTVF, and wSPI upward shifts of the bifurcation values, , as shown in Figure 8, are observed. However, the exact onsets of the different primary bifurcating structures differ, either depending on the particular applied field as well as on .
In absence of a magnetic field (Figure 8(a)) and sufficiently strong counter rotation, , the basic state, CCF, first becomes unstable to a helical solution, SPI, in a supercritical Hopf bifurcation breaking , which results in a pair of symmetrically related, degenerated spiral states, one with left-handed winding and the other with right-handed winding. For considered -parameter range in Figure 8, the bifurcating SPI has an azimuthal wavenumber (or in case of the right-handed SPI). Note that the wavenumber of the primary bifurcating SPI increases with stronger counter-rotating cylinders . On the other hand, for , the basic state loses stability to the toroidally closed TVF. The supercritical pitchfork of revolution bifurcation breaks , and the steady axisymmetric family of solutions are parametrized by their axial location.
Considering a pure axial magnetic field, the scenario remains mainly unchanged (Figure 8(c)); still SPI and TVF appear as primary supercritical flow states with an intersection of the bifurcation thresholds at a specific value . As already seen in Figure 7, increasing field strength in a pure axial field tends to shift the co-dimension -point toward more negative . The same also holds for increasing in a pure transversal field, with significant minor effect on variation. Thus, the magnetic fields tend to render the corresponding basic states more unstable to (w)TVF and more stable to (w)SPI, respectively.
Having a field with finite transversal component, either pure transversal (Figure 8(b)) or oblique orientated (Figure 8(d)), the primary instabilities, with TVF being replaced by wTVF, and SPI being replaced by wSPI, respectively, just as the basic states were modified from CCF to 2-CCF due to the presence of the magnetic field. Their onset occurs at higher values for any given value compared to the onset of classical TVF and SPI in the absence of a magnetic field. Thus, the magnetic fields alter the basic states and make them more robust to instabilities. The level of stabilization is greater for a pure axial field compared to a pure transversal field, but strongest, when an oblique field is imposed (bifurcation values grow with field parameters ).
An oblique magnetic field results in the strongest upward shift of bifurcation values , and also, this shift depends on , which interestingly is largest about , outer cylinder at rest. Furthermore, the topological different flow structures of (w)TVF and (w)SPI are shifted about the same amplitude, with a slightly lager effect on helical (w)SPI for the considered diagram. This should be kept in mind regarding later consideration involving field modulation via internal dependence, presented in Section 5.
So, while a pure axial fields shift the bifurcation onsets more strongly (i.e. to larger values ) than pure transversal ones (Figure 8), the latter one has a stronger influence on the nonlinear spatio-temporal properties and dynamics of the bifurcating vortex structures (Figure 6). Combining both portions to an oblique field enforces both effects. One finds either larger shifts as well as stronger modulated flow structures (Figure 6(e,f)).
An external applied magnetic field (independent of its orientation) stabilizes the CCF (2-CCF) basic state: for a given value of the outer Reynolds number , the bifurcation thresholds for vortex structures are shifted to higher values of the inner Reynolds number . This holds likewise for toroidally closed (w)TVF, as well for helical (w)SPI. Thereby, these shifts are typically linear in the squared field parameters or , respectively. Moreover, stabilization is in general stronger for helical solutions (w)SPI than for toroidally closed ones (w)TVF. Additionally, an external applied magnetic field can, depending on its orientation, change the spatio-temporal structure of the classical TVF and of SPI. The reason is the stimulation of additional modes entering the axial and azimuthal Fourier decomposition of the flow. A pure axial magnetic field keeps the symmetry properties unchanged and does not change the flow structures. It only alter the flow amplitudes, i.e., the magnitude of up-shift in the onsets and magnitude of modes after bifurcation. On the other hand, as soon as a finite transversal field component is present (pure transversal or oblique field), all flow structures become always 3-dimensional and therefore qualitatively different to the classical TVF and SPI states. In particular, they are wavy-like modulated and the pure structures do not exist anymore. Such a field component breaks the system symmetry and therefore alters either basic state (CCF changes to 2-CCF) and supercritical instabilities. As a result, one finds new solutions, field generated, nonrotating wTVF, contrary to the classical rotating ones. The vortex tubes of these wTVF are periodically expanded and constricted in azimuthal -direction, and this deformation pattern is stationary. In general, the bifurcation thresholds for non-axisymmetric, helical (w)SPI are stronger modified in presence of a magnetic field than those for toroidally closed (w)TVF. The upward shift towards larger values of of the former is bigger than for the latter. One direct effect is the shift of the co-dimension point toward stronger counter-rotating frequencies. This effect has been found to show in axial, transversal, and oblique magnetic fields [6, 9].
Finally it is worth to mention that the magnetic field (transversal or oblique field) generated wTVF differ crucially from the classic wTVF [20, 33, 35, 45] that bifurcates secondary out of TVF at relatively high in absence of a magnetic field. The present generated wTVF arises via a primary bifurcation directly out of the 2-CCF basic state.
4. Agglomeration and elongational flow effects
4.1 Introduction and motivation
Aside the general difficulties to incorporate the magnetization of any magnetic field into the governing equations of motion, it is also crucial to consider the specific properties of the magnetic particles. However, most mathematical models describing the flow of complex magnetic fluids typically assume noninteracting magnetic particles with a small volume or only point-size objects. However, real ferrofluids consist of a suspension of particles with a finite size in an almost ellipsoid shape. Moreover, they involve particle-particle interactions resulting in agglomeration; in particular, they tend to form chains of various lengths. One possibility to include such effects and to come close to the realistic situation for ferrofluids is to consider the effect of elongational flow. Mathematically, such flow is incorporated by the symmetric part of the velocity gradient field tensor, which could be scaled by a so-called, material dependent, transport coefficient [10, 37, 38]. As discussed in the previous section, magnetic fields tend to change the bifurcation threshold of the supercritical unstable flows and, depending on their orientation, resulting in structural modifications. Consider elongational flow, these modifications are expected to change the obtained states at least qualitatively.
4.2 Modified internal magnetic field
In order to consider such elongational flow (i.e. agglomeration, chain formation, etc.), one has to determine the relationship between the magnetization , the magnetic field , and the velocity . One possibility is to consider an additional dependence of the magnetization on the symmetric part of the velocity gradient [10, 38]. Thus, the magnetization (4) becomes modified to
Now, using the latest modified magnetization (9), the magnetization part in (1) can be eliminated, similar to previous discussion in Section 2.2. We thus have the following ferrohydrodynamic equation of motion (including elongational flow effects) :
where is the dynamic pressure incorporating all magnetic terms which can be written as gradients, i.e., and . See also (5) for comparison without considered elongational flow.
Assuming that the internal magnetic field is equal to the external imposed magnetic field (it is known as a leading-order approximation , see also following section 5) which is sufficiently good for a ‘first’ numerical investigation for the effect of elongational flow. Therefore, (10) can be simplified:
In this approach, the magnetic field and all the magnetic properties of the ferrofluid could be influenced by the velocity field, the transport coefficient , and the magnetic field Niklas parameters and as described before (7). However, it is worth to mention that in this approach, the material dependent transport coefficient is a parameter , which can be scaled by the term describing the elongational flow and is independent of . Thus, it only appears in combination with the symmetric component of the velocity field tensor. However, real ferrofluids show dependence in the microscopic aspect of the dynamics of ferrofluids with chains or nonspherical particles .
4.3 Linear stability behavior and analysis
Before we come to the influence of onto the fully nonlinear Eqs. (11), it is worth to have a look at the linear marginal stability threshold of the different flow structures. Therefore, in the following, we first investigate the linear growth behavior of either stationary axisymmetric (TVF) and nonaxisymmetric (SPI) oscillatory vortex flow of a ferrofluid in the TCS that is placed in homogeneous axial magnetic fields (Figure 1). In the literature [4, 5, 7, 40, 41, 42], one can find many theoretical works that analyze (via linear stability analysis) the influence of rotational symmetric magnetic fields, i.e., axial, azimuthal, and radial ones on the flow of a ferrofluid in the TCS. However, for a symmetry breaking (e.g., transverse), magnetic field such linear stability analysis is not known for the corresponding basic state at such a field configuration. For a detailed description regarding the linearization around the CCF and solution of the linearized NSE, we refer to the Appendix in .
4.3.1 Marginal stability thresholds
In order to discuss how the transport coefficient influences the growth of and vortex perturbations, we determine the stability of the CCF basic state against these perturbations, considering a magnetic field , applied in pure axial direction.
Figure 9 presents the bifurcation thresholds in the diagram for either axisymmetric, , and nonaxisymmetric, , vortex flow in magnetic fields at (a,b) and (c) for two different axial wavenumbers. Note that the representative axial wavenumber chosen in (a) is as detected in experiments ; (b) . Insets in Figure 9(b,c) show corresponding SPI frequencies at the bifurcation thresholds. As already discussed in Section 3.3.4, the CCF basic state is stabilized against the two types of vortex perturbations in any magnetic field (the lowest thick solid curve in each plot in Figure 9 refers to the case without any magnetic field H = 0 (c.f. Figure 8(a) for non-linear calculation)). Consider elongational flow (), the basic state becomes destabilized in comparison with the case . Regarding Figure 9(a,b), both bifurcation thresholds for and vortices are shifted to lower values of . Thus, for the axial wavenumber of , the term reduces the general stabilization effect caused by an applied magnetic field. For parameters as presented in Figure 9(a,b), this holds for the whole range of presented , even when the changes of the stability boundaries are quite weak, in particular for corotating cylinders. It is important to mention that it never over-compensate the field induced stabilization. Figure 9(c) illustrates in general a strong parameter dependence of the elongational flow effect. While at for TVF and for SPI, increasing also has destabilizing effect, and for corresponding larger , the effect is just opposite. Increasing even enforce the stabilization due to the applied magnetic field.
It is worth to mention that, in contrast to the stabilization of the CCF state by a magnetic field, the -induced modifications of the linear growth of vortices depend significantly on their axial wavenumber as will be discussed below.
4.3.2 Magnetic field dependence of thresholds
Figure 10(I) illustrates the variation of the bifurcation thresholds (TVF) and for (SPI) with the magnetic field , incorporating the elongational flow effect. The top row of figures refers to , and the bottom one to and wavenumbers are (left) and (right), respectively. Ignoring the effect at small , all thresholds increase linearly with . The slopes are given by and vary slightly either with and k. For outer cylinder at rest, , (Figure 10(I)(a)) the slopes of the and curves are comparable, they differ significantly for counter-rotating cylinders, (Figure 10(I)(b)). For the latter, this results in intersections of the and stability boundaries. Such intersections have been observed also in experiments and also in full nonlinear simulations  with .
In general, modifications of the field dependence of the bifurcation thresholds due to tend to increase, when the cylinders are stronger counter-rotating (Figure 10(I)). becomes more negative, and thus, the strain increases. On the other side, they also depend on the axial wavenumber (see also Section 4.3.4). Considering fixed , the modifications due to increase with increasing magnetic field while remaining qualitatively the same. However, the general tendency visible in Figure 11, considering elongational effect, is to shift the stability boundaries downward in . Concrete amounts depend on the parameters and . Note that this relative small destabilizing elongational effect is always overcompensated by the significant stronger general stabilization effect of the magnetic field itself.
4.3.3 Frequencies of helical SPI states
Instead of looking at the growth rates—the real part of the eigenvalue of these solutions (previous Sections), one can also consider the marginal spiral frequency —the imaginary part of the marginal eigenvalue at the bifurcation threshold of (SPI) vortex flow. Figure 10(II) shows the frequency, corresponding to the bifurcation thresholds presented in Figure 10(I). Main effect is the increase of the SPI frequencies with the field , accordingly to the increase of onset Reynolds numbers with (Figure 10(I)). Thus, the threshold frequencies are larger for than for . In general, the effect induced by elongational flow is minor, significant smaller, and only secondary. Analog to the slightly down shift in the onsets (Figure 10(I)) also the SPI frequencies are slightly reduced (Figure 10(II)). Strong counter-rotating cylinders reduce in general the frequency for finite (Figure 10(II)), while for larger wavenumbers, a finite elongational flow at it can be slightly decreased.
A general observation is that all modifications of the spiral frequencies due to finite are most pronounced for the smaller wavenumbers (here in Figure 10) in counter-rotating cylinders. The field dependence is virtually not much modified due to variations in , and the growth rate of the imaginary part of the marginal eigenvalue with increasing is quite similar to that of its real part.
4.3.4 Axial wavenumber dependence
Following, we will first discuss the situation for a (moderately) larger wavenumber, taking as one specific, representative example. For larger value (Figure 9(c)), the situation becomes more complicate. Incorporating the elongational flow scaled by the parameter increases and decreases the growth rate, with respect to , and thus shifts the stability boundaries, up or down, depending on .
Figure 11 illustrates the relation between the wavenumber dependence of the stability boundaries and of the spiral frequencies. This is of particular interest in experiments, since the wavenumbers of some vortex structures show a strong variation when changing the magnetic field [9, 44]. Reindl et al.  also observed hysteresis between vortex flows with different when increasing and decreasing the Reynolds numbers . The bifurcation thresholds (Figure 11, top row and the bottom row ; the (axial) magnetic field is fixed at ) for and vortex flow structures in the diagram change when the elongational term is considered in the linearized ferrofluid equations . Right column of Figure 11(2) presents the wavenumber dependence of the corresponding marginal spiral frequencies at the onsets for SPI.
Typically, the thresholds for (in Figure 11 the case of , lines with squares) are shifted downward in at smaller wavenumbers and upward at larger . Resulting in a fixed magnetic field, the elongational effect destabilizes (stabilizes) the CCF state against growth of vortices with small (large) wavenumbers, either for or perturbations. Consequently, the stability onsets cross for different values of (, in Figure 11) at a specific value of the wavenumber.
It is worth to mention that the crossover values of for and perturbations also depend sensitive on other the control parameters, e.g., . Based on the observations in Figure 11, it is fair to assume that, depending on the wavenumber , the -point (Section 3.3.4) will change.
Similar to the stability thresholds, also the spiral frequencies (Figure 11(2)) increase with increasing when is large and decrease for smaller k as a result of switching on the elongational effect. Thereby, the crossing wavenumber, , separating the increase and decrease in is slightly smaller than the one for crossing the marginal thresholds (Figure 11(a1,b1)). Following the speculation by Odenbach and Müller  on the physical origin of the elongational effect, one can give a reasonable explanation for such an observed wavenumber dependence of the effect on the growth rates of vortex flow. In , the authors argue that the microscopic origin of a finite might be attributed to the finite asphericity of the colloids, i.e., the presence of (short) particle chains in the ferrofluid. Small axial wavenumber will allow these chains more easily to remain aligned in the direction of the magnetic field in vortex flows instead in a flow with large axial wavenumber and large azimuthal vorticity. Larger wavenumber means smaller wavelength and therefore more higher probability to unalign in the given field. Thus, since the magneto-rotational dissipation in the latter flow is larger than in the former one, it requires larger centrifugal forces, i.e., larger values of , to drive the growth of a large flow. However, it is important to state that this argumentation also holds some weakness: In the presence of chains, one could expect also for small vortices an increase of the threshold Reynolds number . On the contrary, incorporating the elongational term in the magnetization balance changes the momentum balance of the vortex flow such that the growth of vortices is enhanced for (left in Figure 10) and reduced for (right in Figure 10) relative to the reference case of .
4.4 Nonlinear analysis
4.4.1 Bifurcation thresholds
Following, we will consider the full nonlinear ferrohydrodynamical equation of motions incorporating elongational flow effects (11) in order to investigate the influence of a finite transport coefficient at different applied magnetic fields.
The general modification in the bifurcation threshold of primary instabilities ((w)TVF) and ((w)SPI) due to finite values remains qualitative as detected and described before in the linear stability analysis in pure axial field. However, the absolute values are slightly different. A direct comparison for axial field (Figures 9-11) results in variation about one to two percent between the calculated onsets using either the linear analysis or full nonlinear equations . While the different field orientations result in different magnitudes of stabilization of the basic states CCF and 2-CCF, respectively, as discussed in Section 3.3.4, a finite value does not depend on different field orientations. The variation effect with is almost identical for all considered field configuration. However, in general, the modifications are slightly larger under oblique magnetic fields. Depending on other system parameters, e.g., wavenumber , cylinder rotation speeds , the effect is either stabilizing or destabilizing with respect to the situation (Figure 10(c) and Figure 11). Considering the effect of elongational flow, the critical bifurcating point of primary centrifugal instability will be shifted either up or down. As detected in the linear analysis, the potential destabilizing effect of never overcomes the general stabilizing effect of the external applied magnetic field, i.e., comparing and any value .
4.4.2 Flow structure modifications
Aside the modification of the primary stability thresholds, there are further flow structural changes/modifications which can be observed for finite value . Figure 11 shows, for different field configurations T: , A: , O: , how the maxima of vorticity vary for either the full flow structure (Figure 12(a)), and reduced 2-fold subspace (Figure 12(b)) varies with for the basic state configuration . Remember, that only for , one has the classical CCF, and for any , a modified basic state is present [6, 9, 37] (i.e., symmetry breaking effect of transversal field). Although for a given configuration (A, T, O), the absolute maxima of these values are significantly different, and their relative differences scale is linear with starting at zero. Lines in Figure 12 are calculated by linear regression fitting to the numerical data points. The effect of is decoupled from the magnetic field configuration and with this the considered flow structure.
Either for classical “pure” CCF or field modified 2-CCF, the variation in grows linear with (Figure 12(a)) (note the significant smaller amplitude in the subspace). Further confirmation for this is the fact that an analog linear growth can be also found when considering other parameters, at which a supercritical flow state exists . This holds for toroidally closed structures (w)TVF, as well as for helical flow states (w)SPI. Only the absolute values in are significant larger.
It is important to mention that the slopes in Figure 12 (for ) not only depend on the applied field orientation (O) but also depend on the strength of the applied magnetic field. With increasing the magnetic field strength , the slopes become steeper. This scenario is illustrated, exemplary for 2-CCF basic state in transversal field configuration in Figure 13.
Moreover, similar characteristics hold for the different primary bifurcating structures. Figure 14 elucidates this effect for the three different field configurations A, T, and O as indicated (see also Figures 4 and 6 in  for another example considering a transversal magnetic field in finite system configuration). For a given field configuration, the slopes increase with , when increasing the magnetic field strength . In general, slopes are smallest for transversal and largest for oblique fields, respectively. The variation in the slopes is continuous with increasing the field strength, but not linear; for larger field strength, the variation in the slopes becomes smaller.
4.4.3 Wavenumber modification and selection
As seen in the former discussion (section 4.3.2), an elongational flow can have strong effect on the axial wavenumber . Consider the full equations (and periodic boundary conditions), one obtains similar results as presented in Figure 10 for linear analysis of the marginal stability thresholds for TVF and SPI. As described before, the agreement between the results of linear and full equations is very close (they differ less than 2 percent).
However, in order to see such wavenumber modification from another perspective, it makes sense to study a finite system with sufficient large aspect ratio enclosed by fixed end plates (assumed to be stationary) on top and bottom. As in a finite system, the axial wavenumber is natural selected by the system itself (depending on the various system parameters), it is possible to see the direct influence, considering a finite value on to the flow structures and their axial wavenumbers .
Starting with a classical TVF as initial flow state, with vortices, which corresponds to an axial wavenumber in the bulk (illustrated on the most left border in Figure 15), we consider a situation with an applied pure transversal magnetic field which is continuously increased for two values, either ignoring any elongational flow effect, (Figure 14(a)), or considering such effect (Figure 15(b)) (note 0.2 is quite small). In any case, either for and for , by increasing the magnetic-field strength, , the number of vortices is reduced, which leads to an increase in the axial wavelength (i.e. decrease in axial wavenumber ) due to elimination of vortices in the bulk. Therefore, the corresponding axial wavenumber in the bulk becomes reduced. Remember that the initial state is a classical, stationary TVF, which becomes modified to stationary wTVF as soon as . For the field generated wTVF, the wavy-like modulation is not visible in Figure 15. However qualitative, the same scenario also holds for either axial and oblique magnetic fields, with changes in the corresponding parameters at which the wavenumber changes, i.e., vortices disappear.
In general, the exact field strength for vortex elimination and/or the number of destroyed vortices depends on . In the example of Figure 15, the initial flow has 22 vortices with an axial wavenumber . Neglecting elongational effects (Figure 15(a)) until the parameter approximately reaches the value about 0.7, the flow remains stable, and the number of vortices in the flow can be reduced to with . Further increasing to about 0.85, the number of vortices can be more reduced to with . Hereafter, no further changes in the number of vortices n appear, before reaching the boundary threshold, . Consider elongational flow (Figure 15(b)), the behavior of the vortex state is similar to the case neglecting such effects. The flow remains stable before the parameter reaches about 0.75. At the same time, the number of vortices is also reduced in analog manner to with . Hereafter, as before, the number of vortices n remains unchanged until the parameter increases to the boundary threshold, . Consider values , the flow structure (for given parameters) is not affected by the magnetic-field strength. A flow with vortices corresponding to axial wavenumber in the bulk is remaining in the bulk.
An interesting phenomenon, which also has been reported in experimental studies  as in numerical simulations, is the fact that one or two vortex pairs can be eliminated. However so far, there is no physical explanation for this observation/phenomenon. Analog to the presented scenario in Figure 15 for pure transversal magnetic field, one also finds similar reduction scenarios for pure axial and oblique magnetic fields. As to expect, the absolute values of field strength, , at which the elimination of vortices happen is different, depending on the applied field.
Real ferrofluids consist of a suspension of particles with finite size and mainly almost ellipsoid shape, as well as there are particle-particle interactions that tend to form chains of various lengths and tend to agglomerate in general. One possibility in order to make a more realistic approach for ferrofluids and to come close to such a configuration in a real ferrofluids is to consider the effect of elongational flow. Such a flow becomes incorporated by the symmetric part of the velocity gradient field tensor in the nondimensional ferrohydrodynamic equations of motion (11) and scales by a material dependent transport coefficient . By such an assumption, the latter is given by a pure scalar number, describing the strength/influence of all former mentioned properties.
Consider either linear stability analysis or fully nonlinear equations, one finds that incorporating such elongational flow can have either stabilization or destabilization effect (i.e., modification in the supercritical primary bifurcation thresholds) with respect to the reference situation in absence of such flow . The modifications due to finite value are qualitative similar and in the same range for different considered magnetic fields, slightly largest in case of an oblique field compared to pure axial or transversal ones. Typically, the modifications due to are larger for helical, nonaxisymmetric, , (w)SPIs than for toroidally closed, axisymmetric, , (w)TVF. Thus, the regim of primary stable bifurcating (w)TVF increases. This observation is similar and goes in hand with the previously described general stabilization of any applied magnetic field (Section 3). There we saw that the stability thresholds of helical flow states are shifted further than those of toroidal closed flow structures. However, it is important and fundamental to state that the elongational effect is never big enough to over compensate the general, field-induced stabilization. Only the magnitude/amplitude in shift can be reduced. Further, it is worth to mention that linear stability analysis is limited to axial magnetic fields; as for fields with finite transversal component, no basic state can be derived, simulations of full nonlinear equations confirm similar effects. The modifications due to are sensitive to various different system parameters (e.g., Reynolds numbers, radius ratio, etc.), in particular sensitive to the axial wavenumber . Here, smaller are strongly effected than larger ones. Thus, considering finite size TCS, a considered elongational flow results in modifications of flow structures in the sense of changing number of vortices in the bulk, which coincides with a different wavenumber selection. Thus, depending on the particular wavenumber, the presence of any elongational effect can be either stabilizing or destabilizing for the basic state. In finite system, this results in different selection and/or modification of number of vortex pairs within the annulus, depending on the parameter.
Regarding the flow structural properties, a finite transport coefficient, , does not change the qualitative shape of the flow pattern. Only quantitative differences can be observed. Essentially, all structural properties remain as generated/induced due to the external applied magnetic field. Thus for instance, the azimuthal mode-2 symmetry originated in the symmetry-breaking transverse magnetic field is preserved; only the strength of different flow quantities is modified (in general they increase) according to finite . Mainly, the flow states become linearly enforced, e.g., speaking in quantity of the azimuthal vorticity, which holds for both the basic flow (CCF, 2-CCF) and the primary instabilities the supercritical centrifugal unstable flows ((w)TVF, (w)SPI).
5. Modified field dependence - internal magnetization
5.1 Introduction and motivation
Aside the properties and behavior of the magnetic particles itself and their interaction with the applied magnetic field (see last sections), the correct assumption of the applied magnetic field is another crucially point in describing magnetic flows and their dynamics. The frequently used, most common assumption is to consider the internal magnetic field within the magnetic fluid (e.g., a ferrofluid) to be equal to the external applied field. Following, we will see that this is only a leading-order approximation. By accounting for the ferrofluid’s magnetic susceptibility, a uniform externally imposed magnetic field is modified by the presence of the magnetic fluid (ferrofluid) within the annulus. The modification to the magnetic field appears in an radial dependence and their magnitude scales with the susceptibility . To be concrete, such modification to the imposed magnetic field can be substantial, also for ferrofluids typically used in laboratory experiments. These have significant consequences on the structural properties and stability of the basic states, as well as on the supercritical (primary) bifurcating solutions.
5.2 Modified internal magnetic field
As already seen in the previous sections, for solving the equation of motion (1), we have to consider the magnetic field within the annular gap between the cylinders. In the last sections, we used the simplest approach with the assumption to take the magnetic field to be identical to the applied external field [4, 6]. However, this simple approach is only a leading-order approximation, and depending on the magnetic susceptibility of the ferrofluid, the magnetic field in the gap is modified.
Assuming infinitely long cylinders, the magnetic boundary conditions are
at and , where is the homogeneous external applied magnetic field in the absence of the ferrofluid-filled annulus and is the radial component of the magnetization .
The following ansatz satisfies a solenoidal field, :
and then the boundary conditions defining the external field are.
To calculate the four unknown constants from the boundary conditions (12), we need the radial component of the magnetization which results from substituting (13) into the magnetization (3):
where stands for the transverse component of . Using the continuity of the magnetic field condition on the cylinders, the coefficients can be calculated. Substituting them into (13), finally the resulting magnetic field is given by
where . A special case of (15) when . This corresponds to an equilibrium magnetization and has been already observed in an earlier work by Odenbach and Müller . They considered the limit of an equilibrium magnetization and used a similar derivation of the modification of the magnetic field for a ferrofluid between two cylinders.
Based on (15), one can use the following magnetic field in the equation of motion:
the dimensionless scalar parameter
characterizes the strength of the radial field dependence . The ferrohydrodynamical equation of motion (6) and the Niklas parameters and (7) remain unchanged/untouched from such considered radial field dependence.
5.3 Flow structural modifications
5.3.1 Primary instabilities
As we learned in previous sections, a magnetic field with a finite transverse component modifies either basic state or primary bifurcating flow structures in a wavy-like manner. More details of these states have been reported in numerical simulations , for which a homogeneous internal magnetic field equal to the external applied one has been supposed, as well as in real experimental studies . The question now is how does the former derived radial field dependence affects the stability of the basic states (CCF and 2-CCF) and the characteristics of the bifurcating solutions ((w)TVF and (w)SPI).
We begin our discussion by considering a purely axial applied magnetic field (A), with fixed field strength , which leaves the flows, in particular its structural properties unaffected (TVF and SPI). Figure 16 shows the influence of the radial field parameter, , (17) (exemplary chosen (a) , (b) and (c) ), on the bifurcation thresholds for TVF and SPI in an axial magnetic field. As in absence of any field dependence, (Figure 16(a)), the bifurcations continue being supercritical. Main effect on the bifurcation curves is that with increasing , the thresholds for the onset of both TVF and SPI are shifted to higher (Figure 16(b,c)). Thereby, the threshold for the toroidally closed TVF being shifted significantly further (to larger values ). Note the different scaling on the abscissa in Figure 16(c). Aside from the enhanced stabilization of the CCF basic state on top of the field introduced stabilization itself, one observes an important consequence to the relative shifts in the two bifurcation curves. Consequently, the bifurcation curve of TVF is shifted more than the one of SPI, the co-dimension-two point, , is also shifted to more positive (c.f. Figure 15(a,b)). Interestingly, this is just the opposite way of the shift with increasing field strength in a pure axial magnetic field (the same holds for in transversal field), which we saw in Figure 7 with moving the -point to the left toward more negative values in . Consider larger values, e.g., (Figure 15(c)), one sees that the co-dimension-two -point is even shifted to out of the considered parameter space. As a result, the primary instability is always the helical SPI, even with the two cylinders in strong co-rotation. This observation is crucially different from classical TCS, both without magnetic fields and also with assumption of an applied uniform magnetic field. Thus, the radial field dependence, induced by the susceptibility of the ferrofluid-filled annulus, is seen to cause major changes in the quantitative and qualitative characteristics of the flow instabilities.
Consider a transversal magnetic field, field strength (Figure 17) instead of an axial one, the variation by increasing remains virtually and qualitatively the same, aside that now all structures are wavy-like modulated (2-CCF, wTVF, wSPI). One finds the same preference, in the sense of stronger upshifts for toroidally closed wTVF with the same result of a shift in the -point to the right to larger values in . Thus also here, for sufficiently strong , e.g., in Figure 17(c), the helical wSPI is the primary stable bifurcating solution in all presented parameter space. Comparing both, pure axial and pure transversal field (at same field strength), the up-shift, i.e., the stabilization is slightly larger in axial fields. This holds for toroidally closed (w)TVF and helical (w)SPI solutions.
Finally, this effect is even more pronounced when an oblique magnetic field is applied as illustrated in Figure 18 for field strength . Note also the different scale on the ordinate in Figure 17(c) highlighting the stronger shifts due to such field configuration. One can speculate that this enforcement is due to the axial component of the oblique field leading to a base state with having axial shear, and the radial field dependence enhances the component of the 2-CCF base state. The combination of the base state azimuthal shear and this axial shear favors the helical instability. Close to the onset, the variation of the maxima of all flow components is almost linear.
5.3.2 Modified flow structures
Figure 19 illustrates the flow structural properties of wTVF and wSPI in either a transverse magnetic field T (a,b) and an oblique magnetic field O (c,d), both with assumed radial field dependence . Note, the flow structures of TVF and SPI under a pure axial applied magnetic field are not shown, as they virtually do not differ from the ones in absence of a magnetic field. Only the absolute values (e.g. in ) are different. Comparing these flow structures to the ones for cases as earlier presented in Figure 6 (Section 3.3.3), one sees the modulations in all structures to be enhanced/enforced. In general, the waviness (axial variation in azimuthal direction) of all flow structures is enforced/enhanced by the radial dependent magnetic field. However, the field-induced wTVF always remains a stationary, nonrotating, and phase-pinned structure, irrespective of whether the radial field dependence is considered or not. On the other hand, wSPIs bifurcate as degenerated solutions, either as a left- or right-winding SPI, depending on initial conditions. Their corresponding frequencies remain mainly constant over a wide range and do not differ much (about 20% or less) from those of SPI. Comparing the stimulated modes for flow structures when (bottom in Figure 19) to those with (bottom in Figure 6), one sees general larger mode amplitudes in the additional stimulated modes for consideration of an internal field dependence . These larger amplitudes in the field induced modes are also the reason for the increase in waviness.
Applying a magnetic field across a container of ferrofluid changes the ferrofluid’s susceptibility and results in modification of the magnetic field structure within the container. So far, most theories commonly neglect such modification, either for convenience or simplicity, and at the end, there is also possibility of numerical simulations in appropriate time or feasibility at all.
However, it is a matter of fact that an external applied magnetic field is modified, depending on the magnetic susceptibility. Experimental studies [10, 38] confirmed the modifications also for susceptibilities of commonly used ferrofluids. Consider such modifications to the imposed magnetic field effects the basic state, its stability, as well as the primary (supercritical) bifurcating solutions. This holds for any field configuration, with only differences in the strength of modifications, i.e., the stabilization (its magnitude; up-shift, move of the bifurcation thesholds to larger control parameters). On the other hand, the flow structural properties remain qualitative unaffected by such an radial field dependence, only change in quantitative manner. They are determined only by the general kind and orientation of the applied magnetic field. Thus, a pure axial field does not have any effect on the flow structural properties, leaving them as in absence of any field, i.e., pure TVF and pure SPI. As described before, the presence of a finite transversal field component results in a wavy-like modulated flow state. This is independent/untouched if the magnetic field is considered to be homogeneous or inhomogeneous with a radial field dependence. However, consider stronger modifications to the imposed magnetic field, i.e., larger values of the radial field dependence parameter have the effect of further strengthening the already present waviness of the structures. This holds for (w)TVF and (w)SPI alike. An important observation is the different influence of the radial field dependence onto topological closed and helical flow states. In general, the effect of modification in the primary bifurcation thresholds is larger for toroidally closed flow structures compared to helical ones. As a result, their intersection point, i.e., co-dimension -point is moved toward positive , which is just the opposite direction, as it moves with increasing the magnetic field strength (for any given field configuration, e.g. Figure 7). The parameter space, the area for which (w)SPI bifurcate primary stable out of the basic state, is growing, even into region of co-rotating cylinders, i.e. , making wSPI the favorable flow state in the system.
Although there has been significant progress in the understanding of ferrofluidic flows in the past decades, their fully theoretical understanding is still limited. A key reason for this is computational high-expensive simulations, which even increase with continuation in refining the models to make them more realistic/appropriate, e.g., finite size effects, internal field modifications, etc. However, these model improvements are essential and necessary to uncover the full potential of ferrofluids, which already are used in a wide field of applications. The use in the car industry within antishocks to provide adjustable damper settings is probably one of the most prominent examples. However, either experiments and numerics are essential to mutually prove each other and combined to provide new inside of potential applications.
This chapter deals with a rotating ferrofluid between two concentric cylinders, i.e., ferrofluid in Taylor-Couette geometry. Therefor we consider different improvements in the model describing such magnetic particles in a flow under external applied field. Concluding the discussions, the main points can be summarized as follows:
Any applied magnetic field changes the bifurcation thresholds of primary solutions—the thresholds of both primary solutions, TVF and SPI, are shifted to larger parameter values—the basic state becomes stabilized against perturbations.
Magnetic fields with a finite transversal component break the system symmetry and renders all flow states to be inherently 3D. As a result, the pure flow states TVF and SPI cease to exist and are substituted by their wave-like cousins, wTVF and wSPI. Thereby, the generated wTVF differs crucially from the classical ones, which rotate in azimuthal direction. Instead, the magnetic field induced wTVFs are nonrotational, phase-pinned flow solutions and develop belly shape structure at specific azimuthal positions.
Assuming elongational flow, in order to consider finite-size effect of the magnetic particles and their interaction (agglomeration, particle-particle interaction and chain formation procedures), one detects further changes in the bifurcation threshold of the solutions. Also, this can result in further stabilization or destabilization. However, the effect of such elongational flow is never big enough to over-compensate the general, field-induced stabilization. Only the magnitude/amplitude varies. The flow states remain structural as in absence of elongational flow.
Accounting for the changes in ferroluid’s susceptibility in the container due to an external magnetic field, the real internal field can be approximated by . As before the flow, structural properties remain qualitative similar. Bifurcation thresholds are shifted upward, toward larger , whereby toroidally closed (w)TVFs are in general preferred and shifted more than helical (w)SPI. The result is an increase in the regime of primary bifurcating (w)SPI.
Conflict of interest
The author declares no conflict of interest.
A.1 Numerical method
There are various different ways to solve the ferrohydrodynamic equations of motions (Eqs. (5) and (10)), the latter including elongational flow). All here presented results have been obtained by a code (G1D3 [6, 7]), which combines a finite difference method of second order in (r,z) and time (explicit) with spectral decomposition in :
where denotes one of . For the parameter regimes investigated here, provides adequate accuracy. For discretization, a forward time, centered space (FTCS) algorithm is used on staggered grids in the plane following the procedure of Hirt et al. . In particular, a homogeneous grid with discretization length and time steps has been used. Here, defines the time step between two iterations via FTCS algorithm of the system of coupled equations for the amplitudes of the azimuthal normal modes . For diagnostic purposes, the complex mode amplitudes were calculated obtained from a second axial Fourier decomposition:
where is the axial wavenumber.
S. Altmeyer is a Serra Húnter Fellow. This work was supported by the Spanish Government grant FIS2017–85794-P.
Nomenclature and abbreviations
|CCF||Circular Couette flow [basic flow]|
|2-CCF||2-fold CCF [basic flow in transversal field]|
|TVF||Taylor vortex flow|
|SPI||Spiral vortex flow (spiral)|